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Effect of disorder in the charge-density-wave compounds LaTe 1.95 and CeTe 1.95-xSe x (x=0 and 0.16) as revealed by optical spectroscopy

  • Y. Huang
  • , B. F. Hu
  • , T. Dong
  • , A. F. Fang
  • , P. Zheng
  • , N. L. Wang

Research output: Contribution to journalArticlepeer-review

7 Scopus citations

Abstract

We present optical spectroscopy measurements on rare-earth ditelluride single crystals of LaTe 1.95 and CeTe 1.95-xSe x (x=0 and 0.16). The measurements reveal formation of charge-density-wave energy gaps at rather high-energy levels, for example, 2Δ∼8500 cm -1 for LaTe 1.95 and 6800 cm -1 for CeTe 1.95. More strikingly, the study reveals that, different from the rare-earth tritellurides, the Te vacancies and disorder effect play a key role in the low-energy charge excitations of ditelluride systems. Although an eminent peak is observed between 800 and 1500 cm -1 in conductivity spectra for LaTe 1.95, and CeTe 1.95-xSe x (x=0 and 0.16), our analysis indicates that it could not be attributed to the formation of a small energy gap, instead it could be well accounted for by the localization modified Drude model. Our study also indicates that the low-temperature optical spectroscopic features are distinctly different from a semiconducting charge-density-wave (CDW) state with entirely gapped Fermi surfaces.

Original languageEnglish
Article number205123
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume86
Issue number20
DOIs
StatePublished - Nov 20 2012
Externally publishedYes

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