Abstract
We present optical spectroscopy measurements on rare-earth ditelluride single crystals of LaTe 1.95 and CeTe 1.95-xSe x (x=0 and 0.16). The measurements reveal formation of charge-density-wave energy gaps at rather high-energy levels, for example, 2Δ∼8500 cm -1 for LaTe 1.95 and 6800 cm -1 for CeTe 1.95. More strikingly, the study reveals that, different from the rare-earth tritellurides, the Te vacancies and disorder effect play a key role in the low-energy charge excitations of ditelluride systems. Although an eminent peak is observed between 800 and 1500 cm -1 in conductivity spectra for LaTe 1.95, and CeTe 1.95-xSe x (x=0 and 0.16), our analysis indicates that it could not be attributed to the formation of a small energy gap, instead it could be well accounted for by the localization modified Drude model. Our study also indicates that the low-temperature optical spectroscopic features are distinctly different from a semiconducting charge-density-wave (CDW) state with entirely gapped Fermi surfaces.
| Original language | English |
|---|---|
| Article number | 205123 |
| Journal | Physical Review B - Condensed Matter and Materials Physics |
| Volume | 86 |
| Issue number | 20 |
| DOIs | |
| State | Published - Nov 20 2012 |
| Externally published | Yes |
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