From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids

A. V. Malko; A. A. Mikhailovsky; M. A. Petruska; Jennifer Ann Hollingsworth; Han Htoon; M. G. Bawendi; Victor Ivanovich Klimov

doi:10.1063/1.1497708

From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids

A. V. Malko
, A. A. Mikhailovsky
, M. A. Petruska
, Jennifer Ann Hollingsworth
, Han Htoon
, M. G. Bawendi
, Victor Ivanovich Klimov

Los Alamos National Laboratory

Research output: Contribution to journal › Article › peer-review

261 Scopus citations

Abstract

We study different emission regimes in close-packed films of chemically synthesized CdSe nanoparticles [nanocrystal quantum dots (NQDs)]. We observe that the NQD photoluminescence is dominated by excitons and biexcitons, respectively, before and after the threshold for stimulated emission. Furthermore, we demonstrate the regime of microring lasing into sharp, whispering-gallery modes using NQD solids incorporated into microcapillary tubes. This result indicates a feasibility of miniature, solid-state laser devices based on chemically synthesized NQDs.

Original language	English
Pages (from-to)	1303-1305
Number of pages	3
Journal	Applied Physics Letters
Volume	81
Issue number	7
DOIs	https://doi.org/10.1063/1.1497708
State	Published - Aug 12 2002

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@article{196c682216dc4e438c69d81ccd9f9fe2,

title = "From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids",

abstract = "We study different emission regimes in close-packed films of chemically synthesized CdSe nanoparticles [nanocrystal quantum dots (NQDs)]. We observe that the NQD photoluminescence is dominated by excitons and biexcitons, respectively, before and after the threshold for stimulated emission. Furthermore, we demonstrate the regime of microring lasing into sharp, whispering-gallery modes using NQD solids incorporated into microcapillary tubes. This result indicates a feasibility of miniature, solid-state laser devices based on chemically synthesized NQDs.",

author = "Malko, \{A. V.\} and Mikhailovsky, \{A. A.\} and Petruska, \{M. A.\} and Hollingsworth, \{Jennifer Ann\} and Han Htoon and Bawendi, \{M. G.\} and Klimov, \{Victor Ivanovich\}",

year = "2002",

month = aug,

day = "12",

doi = "10.1063/1.1497708",

language = "English",

volume = "81",

pages = "1303--1305",

journal = "Applied Physics Letters",

issn = "0003-6951",

publisher = "American Institute of Physics",

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TY - JOUR

T1 - From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids

AU - Malko, A. V.

AU - Mikhailovsky, A. A.

AU - Petruska, M. A.

AU - Hollingsworth, Jennifer Ann

AU - Htoon, Han

AU - Bawendi, M. G.

AU - Klimov, Victor Ivanovich

PY - 2002/8/12

Y1 - 2002/8/12

N2 - We study different emission regimes in close-packed films of chemically synthesized CdSe nanoparticles [nanocrystal quantum dots (NQDs)]. We observe that the NQD photoluminescence is dominated by excitons and biexcitons, respectively, before and after the threshold for stimulated emission. Furthermore, we demonstrate the regime of microring lasing into sharp, whispering-gallery modes using NQD solids incorporated into microcapillary tubes. This result indicates a feasibility of miniature, solid-state laser devices based on chemically synthesized NQDs.

AB - We study different emission regimes in close-packed films of chemically synthesized CdSe nanoparticles [nanocrystal quantum dots (NQDs)]. We observe that the NQD photoluminescence is dominated by excitons and biexcitons, respectively, before and after the threshold for stimulated emission. Furthermore, we demonstrate the regime of microring lasing into sharp, whispering-gallery modes using NQD solids incorporated into microcapillary tubes. This result indicates a feasibility of miniature, solid-state laser devices based on chemically synthesized NQDs.

UR - https://www.scopus.com/pages/publications/79955997290

U2 - 10.1063/1.1497708

DO - 10.1063/1.1497708

M3 - Article

SN - 0003-6951

VL - 81

SP - 1303

EP - 1305

JO - Applied Physics Letters

JF - Applied Physics Letters

IS - 7

ER -

From amplified spontaneous emission to microring lasing using nanocrystal quantum dot solids

Abstract

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