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Magnetic field induced partially polarized chiral spin liquid in a transition metal dichalcogenide moiré system

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Abstract

As one of the most intriguing states of matter, the chiral spin liquid (CSL) has attracted much scientific interest while its existence and mechanism in crystalline strongly correlated systems remain hotly debated. On the other hand, strong correlation driven emergent phenomena can be realized in twisted transition metal dichalcogenide bilayers with a tremendously tunable large length scale providing a new platform for the emergence of CSLs. We focus on a strongly correlated model relevant to heterobilayer WSe2/MoSe2 and investigate the Mott insulating phase at half filling under an out-of-plane magnetic field. Considering both its orbital and spin Zeeman effects we identify three conventionally ordered phases including a 120∘ Néel phase, a stripe phase, and an up-up-down phase. For intermediate fields an emergent quantum spin liquid phase is identified with partial spin polarization. We further characterize its topological nature as the ν=1/2 Laughlin CSL through the topological entanglement spectrum and quantized spin pumping under spin flux insertion. In addition, we map out the quantum phase diagram for different twisted angles in an experimentally accessible parameter regime.

Original languageEnglish
Article number165109
JournalPhysical Review B - Condensed Matter and Materials Physics
Volume109
Issue number16
DOIs
StatePublished - Apr 15 2024

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