Semiclassical simulations of multidimensional Raman echoes

Shaul Mukamel; Andrei Piryatinski; Vladimir Chernyak

doi:10.1063/1.478030

Semiclassical simulations of multidimensional Raman echoes

Shaul Mukamel
, Andrei Piryatinski
, Vladimir Chernyak

Research output: Contribution to journal › Article › peer-review

33 Scopus citations

Abstract

A high-temperature and a weak-nonlinearity (low-temperature) semiclassical expansion are developed for computing two-dimensional vibrational Raman spectroscopies, and applied to an exactly solvable Brownian-oscillator model. The origin of photon echoes is discussed using phase-space-wave-packets. Impulsive and semi-impulsive echoes are shown to satisfy different phase-matching conditions, and are generated in different directions.

Original language	English
Pages (from-to)	1711-1725
Number of pages	15
Journal	Journal of Chemical Physics
Volume	110
Issue number	3
DOIs	https://doi.org/10.1063/1.478030
State	Published - Jan 15 1999
Externally published	Yes

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title = "Semiclassical simulations of multidimensional Raman echoes",

abstract = "A high-temperature and a weak-nonlinearity (low-temperature) semiclassical expansion are developed for computing two-dimensional vibrational Raman spectroscopies, and applied to an exactly solvable Brownian-oscillator model. The origin of photon echoes is discussed using phase-space-wave-packets. Impulsive and semi-impulsive echoes are shown to satisfy different phase-matching conditions, and are generated in different directions.",

author = "Shaul Mukamel and Andrei Piryatinski and Vladimir Chernyak",

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AU - Mukamel, Shaul

AU - Piryatinski, Andrei

AU - Chernyak, Vladimir

PY - 1999/1/15

Y1 - 1999/1/15

N2 - A high-temperature and a weak-nonlinearity (low-temperature) semiclassical expansion are developed for computing two-dimensional vibrational Raman spectroscopies, and applied to an exactly solvable Brownian-oscillator model. The origin of photon echoes is discussed using phase-space-wave-packets. Impulsive and semi-impulsive echoes are shown to satisfy different phase-matching conditions, and are generated in different directions.

AB - A high-temperature and a weak-nonlinearity (low-temperature) semiclassical expansion are developed for computing two-dimensional vibrational Raman spectroscopies, and applied to an exactly solvable Brownian-oscillator model. The origin of photon echoes is discussed using phase-space-wave-packets. Impulsive and semi-impulsive echoes are shown to satisfy different phase-matching conditions, and are generated in different directions.

UR - https://www.scopus.com/pages/publications/0033555044

U2 - 10.1063/1.478030

DO - 10.1063/1.478030

M3 - Article

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VL - 110

SP - 1711

EP - 1725

JO - Journal of Chemical Physics

JF - Journal of Chemical Physics

IS - 3

ER -

Semiclassical simulations of multidimensional Raman echoes

Abstract

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