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Stimulated X-Ray Raman scattering with free-electron laser sources

  • N. Rohringer
  • , V. Kimberg
  • , C. Weninger
  • , A. Sanchez-Gonzalez
  • , A. Lutman
  • , T. Maxwell
  • , C. Bostedt
  • , S. Carron Monterro
  • , A. O. Lindahl
  • , M. Ilchen
  • , R. N. Coffee
  • , J. D. Bozek
  • , J. Krzywinski
  • , T. Kierspel
  • , T. Mullins
  • , J. Küpper
  • , B. Erk
  • , D. Rolles
  • , O. D. Mücke
  • , R. A. London
  • M. Purvis, D. Ryan, J. J. Rocca, R. Feifel, R. Squibb, V. Zhaunerchyk, C. Såthe, M. Agåker, M. Mucke, J. Nordgren, J. E. Rubensson

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

4 Scopus citations

Abstract

Stimulated electronic x-ray Raman scattering is the building block for several proposed x-ray pump probe techniques, that would allow the study of electron dynamics at unprecedented timescales.We present high spectral resolution data on stimulated electronic x-ray Raman scattering in a gas sample of neon using a self-amplified spontaneous emission x-ray free-electron laser. Despite the limited spectral coherence and broad bandwidth of these sources, high-resolution spectra can be obtained by statistical methods, opening the path to coherent stimulated x-ray Raman spectroscopy. An extension of these ideas to molecules and the results of a recent experiment in CO are discussed.

Original languageEnglish
Title of host publicationX-Ray Lasers 2014 - Proceedings of the 14th International Conference on X-Ray Lasers
EditorsJorge Rocca, Carmen Menoni, Mario Marconi
PublisherUnknown Publisher
Pages201-207
Number of pages7
ISBN (Print)9783319195209
DOIs
StatePublished - Jan 1 2016
Externally publishedYes
Event14th International Conference on X-Ray Lasers, 2014 -
Duration: Jan 1 2016 → …

Publication series

NameSpringer Proceedings in Physics
Volume169
ISSN (Print)0930-8989
ISSN (Electronic)1867-4941

Conference

Conference14th International Conference on X-Ray Lasers, 2014
Period01/1/16 → …

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