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Surface plasmon polariton enhanced upconversion in rare earth doped nano crystals on plasmonic substrates

  • Amy Hor
  • , Quocanh Luu
  • , Jon Fisher
  • , Ting Shan Luk
  • , Mahdi Baroughi
  • , P. Stanley May
  • , Steve Smith

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution

1 Scopus citations

Abstract

Plasmonic enhancement of near infra-red to visible upconversion could potentially yield high-efficiency spectral converters for solar cells. We use spectroscopic imaging to investigate the intensity enhancement and modification of radiative rates of infra-red to visible upconversion from rare-earth doped nanoparticles (NaYF4:Yb:Er[Tm]) supported on substrates designed to support a surface plasmon polariton at frequencies which are near-resonant with the rare-earth sensitizer (Yb3+) absorption. Using spatially-resolved spectroscopic imaging, we directly observe a systematic enhancement in the efficiency of upconversion associated with the interaction of the co-doped nano-particles with the plasmonic substrates. Spectrally resolved reflectivity and time-resolved luminescence decay measurements support our interpretation.
Original languageEnglish
Title of host publication2014 IEEE 40th Photovoltaic Specialist Conference, PVSC 2014
Pages2270-2272
Number of pages3
DOIs
StatePublished - Oct 15 2014
Externally publishedYes

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